Direct Measurement of the Intrinsic Electric Dipole Moment in Pear-Shaped Thorium-228

The intrinsic dipole moment of Th-228 is reported, from which the degree of the nucleus's octupole deformation is estimated, suggesting that Th-229 and Pa-229 may be suitable candidates for the search for a permanent atomic electric dipole moment. Atomic nuclei with certain combinations of proton and neutron numbers can adopt reflection-asymmetric or octupole-deformed shapes at low excitation energy. These nuclei present a promising avenue in the search for a permanent atomic electric dipole moment-the existence of which has implications for physics beyond the Standard Model of particle physics. Theoretical studies have suggested that certain thorium isotopes may have large octupole deformation. However, due to experimental challenges, the extent of the octupole collectivity in the low-energy states in these thorium nuclei has not yet been demonstrated. Here, we report measurements of the lifetimes of low-energy states in Th-228 (Z = 90) with a direct electronic fast-timing technique, the mirror symmetric centroid difference method. From lifetime measurements of the low-lying J(pi) = 1(-) and J(pi) = 3(-) states, the E1 transition probability rates and the intrinsic dipole moment are determined. The results are in agreement with those of previous theoretical calculations, allowing us to estimate the extent of the octupole deformation of Th-228. This study indicates that the nuclei Th-229 and Pa-229 (Z = 91) may be good candidates for the search for a permanent atomic electric dipole moment.